Investigating products of titanium dissolution in the presence of fluoride ions with dual dynamic voltammetry
DOI:
https://doi.org/10.5599/jese.502Keywords:
Rotating ring–disk electrodes, electrochemical map, cyclic voltammetry, dental implant materials, corrosionAbstract
Products of titanium dissolution in the active state are investigated in fluoride containing 1 M H2SO4 solutions. The novel method of dual dynamic voltammetry, applied to Ti disk/Pt ring rotating ring–disk electrodes, is utilized for the simultaneous detection of different dissolution products. Potential regions where certain products (primarily, TiIII and H2) are formed are identified by a 3D electrochemical map constructed based on the ring–disk electrode measurements. Besides dissolution in the form of TiIII species and hydrogen evolution, the formation and prompt oxidation of TiII can also be presumed under the applied conditions.
Downloads
References
M. Stern, H. Wissenberg Journal of The Electrochemical Society 106 (1959) 755-759
J. J. Kelly, Electrochimica Acta 24 (1979) 1273-1282
D. J. Blackwood, L. M. Peter, D. E. Williams, Electrochimica Acta 33 (1988) 1143-1149
M. J. Mandry, G. Rosenblatt, Journal of The Electrochemical Society 119 (1972) 29-33
Z. B. Wang, H. X. Hu, C. B. Liu, Y. G. Zheng, Electrochimica Acta 135 (2014) 526-535
R. D. Armstrong, J. A. Harrison, H. R. Thirsk, R. Whitfield, Journal of The Electrochemical Society 117 (1970) 1003-1006
E. J. Kelly, Journal of The Electrochemical Society: Electrochemical Science and Technology 123 (1976) 162-170
J. A. Harrison, D. E. Williams, Electrochimica Acta 27 (1982) 891-895
W. B. Utomo, S. W. Donne, Electrochimica Acta 51 (2006) 3338-3345
D. Devilliers, M. T. Dinh, E. Mahé, D. Krulic, N. Larabi, N. Fatouros, Journal of New Materials for Electrochemical Systems 9 (2006) 221-232
E. J. Kelly, H. R. Bronstein, Journal of The Electrochemical Society: Electrochemical Science and Technology 131 (1984) 2232-2238
W. Wilhelmsen, A.P. Grande, Electrochimica Acta 32 (1987) 1469-1474
D.-S. Kong, Langmuir 24 (2008) 5324-5331
M. S. Amrutha, F. Fasmin, S. Ramanathan, Journal of The Electrochemical Society 164 (2017) H188-H197
D. J. Wever, A. G. Veldhuizen, J. de Vries, H. J. Busscher, D. R. A. Uges, J. R. van Horn, Biomaterials 19 (1998) 761-769
J. E. G. González, J. C. Mirza-Rosca, Journal of Electroanalytical Chemistry 471 (1999) 109-115
M. Nakagawa, S. Matsuya, K. Udoh, Dental Materials Journal 20 (2001) 305-314
N. Schiff, B. Grosgogeat, M. Lissac, F. Dalard, Biomaterials 23 (2002) 1995-2002
A. S. Mogoda, Y. H. Ahmad, W. A. Badawy, Journal of Applied Electrochemistry 34 (2004) 873-878
B. Lindholm-Sethson, B. I. Ardlin, Journal of Biomedical Materials Research Part A 86A (2008) 149-159
V. A. Alves, R. Q. Reis, I. C. B. Santos, D. G. Souza, T. de F. Gonçalves, M. A. Pereira-da-Silva, A. Rossi, L. A. da Silva, Corrosion Science 51 (2009) 2473-2482
J. C. M. Souza,S. L. Barbosa, E. A. Ariza, M. Henriques, W. Teughels, P. Ponthiaux, J.-P. Celis, L. A. Rocha, Materials Science and Engineering C 47 (2015) 384-393
S. Vesztergom, M. Ujvári, G. G. Láng, Electrochemistry Communications 13 (2011) 378-381
S. Vesztergom, M. Ujvári, G. G. Láng, Electrochemistry Communications 19 (2012) 1-4
N. Kovács, M. Ujvári, G. G. Láng, P. Broekmann, S. Vesztergom, Instrumentation Science and Technology 43 (2015) 633-648
S. Vesztergom, M. Ujvári, G. G. Láng, Electrochimica Acta 110 (2013) 49-55
S. Vesztergom, N. Kovács, M. Ujvári, G. G. Láng, tm - Technisches Messen 84 (2017) 683-696
S. Vesztergom, in Reference Module in Chemistry, Molecular Sciences and Chemical Engineering, Elsevier, Amsterdam, Netherlands, 2018, chapter id. 13563-2
S. Vesztergom, M. Ujvári, G.G. Láng, in Voltammetry: Theory, Types and Applications, Y. Saito, T. Kikuchi, Eds., Nova Science Publishers, New York, USA, 2013, p. 249
S. Schuldiner Journal of The Electrochemical Society 115 (1968) 362-365
J. Bao, D. D. Macdonald, Journal of Electroanalytical Chemistry 600 (2007) 205-216
A. E. von Mengershausen, N. V. Almeida, M. N. Barzola, J. O. Zerbino, S. M. Esquenoni, M. G. Sustersic, Green and Sustainable Chemistry 4 (2014) 55-59
Downloads
Published
How to Cite
Issue
Section
License
Articles are published under the terms and conditions of the
Creative Commons Attribution license 4.0 International.